Bolongaro et al. (2025): Life-Cycle Assessment of Solid Calcium-Looping Direct Air Capture and Its Synergistic Dual Use for Net-Negative Cement

Vittoria Bolongaro, David Yang Shu, Noah McQueen and André Bardow, IN: ChemRXiv, https://doi.org/10.26434/chemrxiv-2025-8zjlg-v2

Calcium-looping direct air carbon capture and storage (DACCS) is a mature technology positioned for gigatonne-scale carbon dioxide removal (CDR). However, a holistic assessment of its system-wide environmental performance and large-scale implications remains critically absent. Here, the authors present a prospective life cycle assessment (LCA) of megatonne-scale calcium-looping DACCS systems under projected 2050 energy scenarios, evaluating CO₂ removal alongside 18 other environmental impact categories.

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