Wang et al. (2024): Amine/vermiculite composite aerogels fabricated by polyethyleneimine-induced vermiculite nanosheet gelation for efficient direct air capture
Shuai Wang, Huilian Sun, Jie Wang, Cong Chen, Lanlan Jiang, Yi Zhang, Yu Liu, Yongchen Song, Zheng Ling IN: Chemical Engineering Journal, 498, 155478, https://doi.org/10.1016/j.cej.2024.155478
In this study, a simple, cost-effective, and environmentally friendly method for fabricating amine/vermiculite composite aerogels is proposed for capturing CO2 from ambient air. Natural two-dimensional material, vermiculite nanosheets with exposed surface and intrinsic negative charge, was utilized as the the building blocks for fabricating aerogel as solid amine adsorbents, via the fast gelatin between vermiculite and amine, significantly reducing the cost of adsorbent preparation while achieving promising CO2 capture capability. The effects of amine loading, amine molecular weight, and porosity on CO2 capture capacity and amine efficiency were investigated.